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Towering wildfire clouds have big impacts on the stratosphere

Images of vast clouds of wildfire smoke towering into the sky have become all too familiar from recent active fire years across the western United States and Australia. Now, a team of atmospheric scientists led by NOAA has demonstrated these big vertical plumes of wildfire smoke have a major long term impact on the stratosphere - and climate. 

Fire-triggered thunderstorms, called pyrocumulonimbus or pyroCbs, are generated when the intense heat of a wildfire triggers a huge thunderstorm that carries smoke into the stratosphere, five to seven miles above the surface. In 2017, the flight path of a NASA airborne mission to study the background atmosphere over the remote oceans, the Atmospheric Tomography mission (ATom), intersected with smoke from the largest pyroCb event observed in the satellite era to that date over the Pacific Northwest. The smoke injection was so large that remote sensing instruments around the globe monitored it for more than eight months. Measurements showed that it and several additional Northern Hemisphere pyroCb events that year dominated contributions of black carbon and organic carbon to the lower stratosphere, the net effect of which cooled the planet.

The results have been published in the journal Science.

“These fire clouds are growing larger and more frequent – witness record-breaking events in 2017, 2019 and 2020,” said NOAA scientist Joshua Schwarz. “Their recent impacts on the stratosphere have been impressive. Now we’ve learned how to track those impacts over longer time periods than we previously recognized were significant. This means we’ll now be able to track changes in their impacts as the climate evolves.”

Scientists are interested in learning more about pyroCbs because their smoke lingers in the atmosphere longer than that from typical fires, affecting climate on a different scale. Schwarz, a research physicist with the Chemical Sciences Laboratory and co-author on the paper, added that the findings also provide insights about the behavior of aerosols from volcanoes, aviation, or potential future solar geoengineering efforts. 

Yet critical measurements of these huge clouds have been extremely limited because of their highly episodic nature, and the logistical challenges of getting scientific instruments airborne and into the smoke on short notice. As a result, the distribution and duration of smoke from these events is poorly known, as is the impact on climate and stratospheric aerosol chemistry, including the ozone layer. 

One surprising finding was the discovery of an extremely thick coating on black carbon particles generated by wildfires. 

"We spent weeks analyzing individual particle data to verify that this was a real signal, and not generated by some fault in the data processing,” said former CIRES scientist and lead author Joe Katich, who now works for Ball Aerospace. 

A second NOAA-NASA airborne mission, FIREX-AQ, provided direct sampling of hours old pyroCb smoke from the Williams Flats fire in 2019. Analysis of black carbon from that fire gave them more confidence about their conclusions drawn from the 2017 smoke.

The thick coating on black carbon, along with its size, and mass, was a remarkably stable feature of pyroCb smoke that researchers realized could be used to “fingerprint” these particles in the lower stratosphere. Using these fingerprints, they re-examined data from a total of 12 airborne mission datasets going back to 2006 in both hemispheres to estimate long-term pyroCb influences on the lower stratosphere in our recent climate.

The researchers found that even in those years with relatively few of these pyroCbsbefore more active fire seasons starting in 2020, the impact of smoke was very significant, contributing roughly 20% of all stratospheric black carbon and organic carbon in the lower stratosphere in the previous decade. 

“This gave us a reasonable estimate representing the period before things really started lighting up,” Schwarz said. “We now recognize pyroCb’s longer term influence on the stratosphere. It’s not just an important blip, but a steady state influence that needs to be accounted for.” 

The big picture takeaway? “This is a major win for understanding the stratosphere, which people have a rapidly growing interest in,” Katich added.”PyroCb contributes more to the stratospheric makeup than we thought, acts in different ways than we thought, and sticks around longer than we thought. This finding is important on its own, but will also help us understand the long-term implications of solar geoengineering with aerosols.”

Original source can be found here.

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